TY - JOUR
T1 - Photon-induced near-field electron microscopy (PINEM)
T2 - Theoretical and experimental
AU - Park, Sang Tae
AU - Lin, Milo
AU - Zewail, Ahmed H.
PY - 2010/12
Y1 - 2010/12
N2 - Electron imaging in space and time is achieved in microscopy with timed (near relativistic) electron packets of picometer wavelength coincident with light pulses of femtosecond duration. The photons (with an energy of a few electronvolts) are used to impulsively heat or excite the specimen so that the evolution of structures from their nonequilibrium state can be followed in real time. As such, and at relatively low fluences, there is no interaction between the electrons and the photons; certainly that is the case in vacuum because energy-momentum conservation is not possible. In the presence of nanostructures and at higher fluences, energy-momentum conservation is possible and the electron packet can either gain or lose light quanta. Recently, it was reported that, when only electrons with gained energy are filtered, near-field imaging enables the visualization of nanoscale particles and interfaces with enhanced contrast (Barwick et al 2009 Nature 462 902). To explore a variety of applications, it is important to express, through analytical formulation, the key parameters involved in this photon-induced near-field electron microscopy (PINEM) and to predict the associated phenomena of, e.g., forty-photon absorption by the electron packet. In this paper, we give an account of the theoretical and experimental results of PINEM. In particular, the time-dependent quantum solution for ultrafast electron packets in the nanostructure scattered electromagnetic (near) field is solved in the high kinetic energy limit to obtain the evolution of the incident electron packet into a superposition of discrete momentum wavelets. The characteristic length and time scales of the halo of electron-photon coupling are discussed in the framework of Rayleigh and Mie scatterings, providing the dependence of the PINEM effect on size, polarization, material and spatiotemporal localization. We also provide a simple classical description that is based on features of plasmonics. A major part of this paper is devoted to the comparisons between the theoretical results and the recently obtained experimental findings about the imaging of materials and biological systems.
AB - Electron imaging in space and time is achieved in microscopy with timed (near relativistic) electron packets of picometer wavelength coincident with light pulses of femtosecond duration. The photons (with an energy of a few electronvolts) are used to impulsively heat or excite the specimen so that the evolution of structures from their nonequilibrium state can be followed in real time. As such, and at relatively low fluences, there is no interaction between the electrons and the photons; certainly that is the case in vacuum because energy-momentum conservation is not possible. In the presence of nanostructures and at higher fluences, energy-momentum conservation is possible and the electron packet can either gain or lose light quanta. Recently, it was reported that, when only electrons with gained energy are filtered, near-field imaging enables the visualization of nanoscale particles and interfaces with enhanced contrast (Barwick et al 2009 Nature 462 902). To explore a variety of applications, it is important to express, through analytical formulation, the key parameters involved in this photon-induced near-field electron microscopy (PINEM) and to predict the associated phenomena of, e.g., forty-photon absorption by the electron packet. In this paper, we give an account of the theoretical and experimental results of PINEM. In particular, the time-dependent quantum solution for ultrafast electron packets in the nanostructure scattered electromagnetic (near) field is solved in the high kinetic energy limit to obtain the evolution of the incident electron packet into a superposition of discrete momentum wavelets. The characteristic length and time scales of the halo of electron-photon coupling are discussed in the framework of Rayleigh and Mie scatterings, providing the dependence of the PINEM effect on size, polarization, material and spatiotemporal localization. We also provide a simple classical description that is based on features of plasmonics. A major part of this paper is devoted to the comparisons between the theoretical results and the recently obtained experimental findings about the imaging of materials and biological systems.
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U2 - 10.1088/1367-2630/12/12/123028
DO - 10.1088/1367-2630/12/12/123028
M3 - Article
AN - SCOPUS:78651328576
SN - 1367-2630
VL - 12
JO - New Journal of Physics
JF - New Journal of Physics
M1 - 123028
ER -